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The Journal of chemical physics · 2026

Emergent clusters in strongly confined systems.

СтатьяНазвание и аннотация: Перевод в очереди
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Bethmage Pamud Akalanka, Fish Ryker, Sprinkle Brennan, Driscoll Michelle M

Аннотация

Driven suspensions, where energy is input at a particle scale, are a framework for understanding general principles of out-of-equilibrium organization. A large number of simple interacting units can give rise to non-trivial structure and hierarchy. Rotationally driven colloidal particles are a particularly nice model system for exploring this pattern formation, as the dominant interaction between the particles is hydrodynamic. Here, we use experiments and large-scale simulations to explore how strong confinement alters dynamics and emergent structure at the particle scale in these driven suspensions. Surprisingly, we find that large-scale density fluctuations (many times the particle size) emerge as a result of confinement, and that these density fluctuations sensitively depend on the degree of confinement. We extract a characteristic length scale for these fluctuations, demonstrating that the simulations quantitatively reproduce the experimental pattern. Moreover, we show that these density fluctuations are a result of the large-scale recirculating flow generated by the rotating particles inside a sealed chamber. This surprising result shows that, even when system boundaries are far away, they can cause qualitative changes to mesoscale structure and ordering.

ИП Урсолов Владлен Сергеевич

ИНН 500118482352 · ОГРНИП 314500117700049

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