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DOI 10.1021/acsnano.5c20740

Медицинская библиотека · ACS nano · 2026

Integration of 2D Materials in Radial van der Waals Heterostructure Metasurfaces.

Heimig Connor, Biechteler Jonas, Cruciano Cristina, Genco Armando, Weber Thomas, Hirler Michael, Gryb Dmytro, de S Menezes Leonardo, Valentini Gianluca, Manzoni Cristian, Cerullo Giulio, Maier Stefan A, Antonov Alexander A, Sortino Luca, Tittl Andreas

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Аннотация

Two-dimensional semiconductors, such as monolayer transition metal dichalcogenides (TMD), exhibit strong excitonic transitions at room temperature and offer a platform for exploring light-matter interactions in nanoscale photonic systems. In this work, we demonstrate a compact and polarization-invariant photonic metasurface, fabricated from hexagonal boron-nitride (hBN) and based on radial bound states in the continuum (BIC), which are formed by radially distributed pairs of structurally asymmetric resonators. The metasurface employs multiple symmetry-breaking perturbations to support high-quality (Q) factor resonances within a radial footprint of 4.5 μm - approximately one-sixth of the area of previous hBN BIC metasurface implementations based on large periodic arrays. Compared to these approaches, the radial geometry furthermore achieves sizable Q-factors with a reduced footprint. By integrating the hBN photonic structure with a WS2 monolayer, we observe enhanced photoluminescence when its resonance is spectrally aligned with the exciton resonance, accompanied by signatures of discrete momentum-space patterns that identify the orbital-angular-momentum-carrying ring eigenmodes. These features persist over a wide range of excitation powers and show minimal linewidth broadening, indicating robust and spatially modulated exciton-photon coupling. This work establishes a scalable approach for generating hybrid photonic-excitonic states with momentum-space structure, offering opportunities for exciton localization, valley emission, spatially programmable light-matter interaction in 2D material platforms and compact luminescent devices based on 2D material integrated metasurfaces.

Для цитирования: Heimig Connor, Biechteler Jonas, Cruciano Cristina, Genco Armando, Weber Thomas, Hirler Michael, Gryb Dmytro, de S Menezes Leonardo, Valentini Gianluca, Manzoni Cristian, Cerullo Giulio, Maier Stefan A, Antonov Alexander A, Sortino Luca, Tittl Andreas. Integration of 2D Materials in Radial van der Waals Heterostructure Metasurfaces.. ACS nano. 2026. DOI: 10.1021/acsnano.5c20740.
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