Journal of colloid and interface science · 2026
Independent control of transport and order in a ratcheted colloidal suspension.
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Mandal Sudipta, Chakraborty Dipanjan, Chaudhuri Debasish
Аннотация
We study directed transport in a two-dimensional suspension of repulsively interacting colloids driven by a stochastic asymmetric piecewise-linear flashing ratchet using large-scale molecular dynamics simulations. The driving frequency and the ratchet asymmetry offer two independent ways of controlling the particle current, but they affect the suspension differently. At fixed asymmetry, the current shows a resonance with ratcheting frequency that is set by the collective relaxation dynamics of the interacting particles. The resulting increase in transport is accompanied by structural reorganization and by changes in the population of topological defects, showing density-dependent hexatic and solid-like states, with larger currents generally associated with weaker ordering.By contrast, at fixed frequency, changing the ratchet asymmetry mainly alters the strength of the directed bias and can significantly enhance the current while leaving the hexatic order largely unchanged. Near the equilibrium hexatic-melting regime, this makes it possible to generate substantial directed currents without strongly disrupting sixfold orientational order. These results show that frequency tuning couples transport to structural reorganization, whereas asymmetry tuning primarily controls transport leaving the structure largely unaltered, providing distinct and complementary routes for manipulating transport and order in driven colloidal suspensions.